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Condensed Matter > Superconductivity

arXiv:2309.00261 (cond-mat)
[Submitted on 1 Sep 2023 ]

Title: Suppression of both superconductivity and structural transition in hole-doped MoTe$_2$ induced by Ta substitution

Title: 空穴掺杂MoTe$_2$中由Ta取代引起的超导性和结构相变的抑制

Authors:Siu Tung Lam, K. Y. Yip, Swee K. Goh, Kwing To Lai
Abstract: Type-II Weyl semimetal MoTe$_2$ exhibits a first-order structural transition at $T_s$ $\sim$250~K and superconducts at $T_c$ $\sim$0.1~K at ambient pressure. Both $T_s$ and $T_c$ can be manipulated by several tuning parameters, such as hydrostatic pressure and chemical substitution. It is often reported that suppressing $T_s$ enhances $T_c$, but our study shows a different behaviour when MoTe$_2$ is hole-doped by Ta. When $T_s$ is suppressed by Ta doping, $T_c$ is also suppressed. Our findings suggest that the suppression of $T_s$ does not necessarily enhance superconductivity in MoTe$_2$. By connecting with the findings of electron-doped MoTe$_2$, we argue that varying electron carrier concentration can effectively tune $T_c$. In addition, the Hall coefficient is enhanced around the doping region, where $T_s$ is completely suppressed, suggesting that the critical scattering around the structural transition may also play a role in suppressing $T_c$.
Abstract: Type-II Weyl semimetal MoTe$_2$ exhibits a first-order structural transition at $T_s$ $\sim$ 250~K and superconducts at $T_c$ $\sim$ 0.1~K at ambient pressure. Both $T_s$ and $T_c$ can be manipulated by several tuning parameters, such as hydrostatic pressure and chemical substitution. 经常有报道指出,抑制$T_s$会增强$T_c$,但我们的研究表明,当 MoTe$_2$通过 Ta 掺杂进行空穴掺杂时,表现出不同的行为。 当$T_s$被 Ta 掺杂抑制时,$T_c$也被抑制。 我们的研究结果表明,$T_s$的抑制并不一定增强 MoTe$_2$中的超导性。 通过与电子掺杂 MoTe$_2$的研究结果相结合,我们认为改变电子载流子浓度可以有效调节$T_c$。 此外,在掺杂区域附近霍尔系数增强,其中$T_s$完全被抑制,这表明结构相变附近的临界散射也可能在抑制$T_c$中起到作用。
Subjects: Superconductivity (cond-mat.supr-con) ; Materials Science (cond-mat.mtrl-sci); Strongly Correlated Electrons (cond-mat.str-el)
Cite as: arXiv:2309.00261 [cond-mat.supr-con]
  (or arXiv:2309.00261v1 [cond-mat.supr-con] for this version)
  https://doi.org/10.48550/arXiv.2309.00261
arXiv-issued DOI via DataCite
Journal reference: Phys. Rev. Materials 7, 084802 (2023)
Related DOI: https://doi.org/10.1103/PhysRevMaterials.7.084802
DOI(s) linking to related resources

Submission history

From: Siu Tung Lam [view email]
[v1] Fri, 1 Sep 2023 05:33:26 UTC (2,123 KB)
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