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Condensed Matter > Strongly Correlated Electrons

arXiv:2407.00498 (cond-mat)
[Submitted on 29 Jun 2024 (v1) , last revised 17 Sep 2024 (this version, v3)]

Title: Quantum oscillation study of the large magnetoresistance in Mo substituted WTe$_2$ single crystals

Title: Mo掺杂WTe$_2$单晶中巨大磁阻的量子振荡研究

Authors:Sourabh Barua, M. R. Lees, G. Balakrishnan, P. A. Goddard
Abstract: The list of interesting electrical properties exhibited by transition metal dichalcogenides has grown with the discovery of extremely large magnetoresistance (MR) and type-II Weyl semimetal behaviour in WTe$_2$ and MoTe$_2$. The extremely large MR in WTe$_2$ is still not adequately understood. Here, we systematically study the effect of Mo substitution on the quantum oscillations in the MR in WTe$_2$. The MR decreases with Mo substitution, however, the carrier concentrations extracted from the quantum oscillations show that the charge compensation improves. We believe that earlier interpretations based on the two-band theory, which attribute the decrease in MR to charge imbalance, could be incorrect due to over-parametrization. We attribute the decrease in MR in the presence of charge compensation to a fall in transport mobility, which is evident from the residual resistivity ratio data. The quantum scattering time and the effective masses do not change within experimental errors upon substitution.
Abstract: 过渡金属二硫属化物所表现出的有趣电学性质列表随着在WTe$_2$和 MoTe$_2$中发现极大的磁阻(MR)和 II 型 Weyl 半金属行为而不断增加。WTe$_2$中的极大磁阻现象仍未得到充分理解。在这里,我们系统地研究了钼取代对 WTe$_2$磁阻中量子振荡的影响。磁阻随着钼的取代而减小,然而,从量子振荡中提取的载流子浓度表明,电荷补偿有所改善。我们认为,基于双带理论的早期解释——将磁阻的降低归因于电荷不平衡——由于过度参数化可能是错误的。我们认为,在存在电荷补偿的情况下磁阻的下降应归因于输运迁移率的降低,这可以从残余电阻比数据中看出。量子散射时间和有效质量在实验误差范围内并未因取代而发生变化。
Comments: This revised version includes minor revisions after peer-review
Subjects: Strongly Correlated Electrons (cond-mat.str-el)
Cite as: arXiv:2407.00498 [cond-mat.str-el]
  (or arXiv:2407.00498v3 [cond-mat.str-el] for this version)
  https://doi.org/10.48550/arXiv.2407.00498
arXiv-issued DOI via DataCite
Journal reference: Phys. Rev. B 110 (2024) 155113
Related DOI: https://doi.org/10.1103/PhysRevB.110.155113
DOI(s) linking to related resources

Submission history

From: Sourabh Barua Dr [view email]
[v1] Sat, 29 Jun 2024 17:19:46 UTC (5,420 KB)
[v2] Tue, 2 Jul 2024 11:58:12 UTC (5,420 KB)
[v3] Tue, 17 Sep 2024 05:37:02 UTC (5,443 KB)
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